Quantum network approach to spin interferometry driven by Abelian and non-Abelian fields
Abstract
This work was supported by the Spanish Ministerio de Ciencia, Innovación y Universidades through Projects No. FIS2017-82804-P (A.H., T.B., and D.B.) and No. FIS2017-86478-P (D.F.), and by the Transnational Common Laboratory Quantum – ChemPhys (D.B.).
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PHYSICAL REVIEW B 103, 155419 (2021) Quantum network approach to spin interferometry driven by Abelian and non-Abelian fields A. Hijano ,1,2,3,*T. L. van den Berg ,2,†D. Frustaglia ,4,‡and D. Bercioux 2,5,§ 1Department of Applied Physics II, University of the Basque Country UPV/EHU, Apartado 644, 48080 Bilbao, Spain 2Donostia International Physics Center (DIPC), 20018 Donostia–San Sebastián, Spain 3Centro de Física de Materiales (CFM-MPC) Centro Mixto CSIC-UPV/EHU, E-20018 Donostia-San Sebastián, Spain 4Departamento de Física Aplicada II, Universidad de Sevilla, E-41012 Sevilla, Spain 5IKERBASQUE, Basque Foundation for Science, Plaza Euskadi 5, 48009 Bilbao, Spain (Received 2 February 2021; revised 30 March 2021; accepted 1 April 2021; published 21 April 2021) We present a theory of conducting quantum networks that accounts for Abelian and non-Abelian fields acting on spin carriers. We apply this approach to model the conductance of mesoscopic spin interferometers of different geometry (such as squares and rings), reproducing recent experimental findings in nanostructured InAsGa quantum wells subject to Rashba spin-orbit and Zeeman fields (as, e.g., the manipulation of Aharonov-Casher interference patterns by geometric means). Moreover, by introducing an additional field-texture engineering, we manage to single out a previously unnoticed spin-phase suppression mechanism. We notice that our approach can also be used for the study of complex networks and the spectral properties of closed systems. DOI: 10.1103/PhysRevB.103.155419 I. INTRODUCTION Within the development of mesoscopic physics, coherent spin transport in quantum electronics has attracted a great deal of attention along the past decades [1]. This interest runs from the study of fundamental spin-based phenomena, such as weak antilocalization [2] and geometric/topological spin phases [3,4], to proposals for spintronic applications, such as spin field-effect transistors [5–7], spin filtering [8], spin qubits [9,10], and, more recently, spin-based platforms for topological quantum computing [11]. Additionally, the understanding of quantum phenomena associated to coherent transport can pave the way to enhance and improve the sensibility of nanometer-sized devices [12]. A common ingredient here is the role played by Abelian and non-Abelian phases produced by the carriers’ spin dynamics under the action of magnetic textures originating from either (i) purely magnetic sources, such as micromagnetic arrays leading to inhomogeneous Zeeman coupling [13–16], (ii) purely electric sources, leading to spin-orbit interaction such as Rashba or Dresselhaus coupling [17,18], or (iii) hybrid sources, combining magnetic and spin-orbit fields [19,20]. Most experimental implementations are performed by using materials with strong Rashba spin-orbit coupling (RSOC) such as InAlAs/InGaAs heterostructures, which allow for the electrical control of the RSOC strength via top gates. The recent transport experiments with mesoscopic interferometers performed by Nitta’s group [19–22] showed evidence of electronic wave-function manipulation through both the *[email protected] †tineke.v[email protected]g ‡[email protected] §[email protected] charge and the spin degrees-of-freedom. The charge degreeof-freedom responds to magnetic fluxes whereas the spin reacts to the RSOC (and to additional Zeeman fields). The orbital coupling to magnetic fields gives rise to the AharonovBohm effect [23] and the spin coupling to electric fields is responsible for the Aharonov-Casher effect [24] | the electromagnetic dual of the previous one. Experiments reporting the observation of the Aharonov-Casher effect in mesoscopic systems were carried out in HgTe heterostructures [25], three-dimensional topological insulators [26], and Josephson junction circuits [27], whereas the Aharonov-Bohm effect has been extensively observed in metallic rings [28], p-type GaAs heterostructures [29], and carbon nanotubes, [30] among others. The modeling of spin-dependent transport in mesoscopic systems can demand significant numerical efforts. The most popular technique has been the recursive construction of Green’s functions from tight-binding Hamiltonians [31,32], a very reliable method which sometimes turns out to be expensive in computational terms. More recently, the development of the open-source KWANT code [33], based on a wave-function scattering approach, represented a major step towards computational efficiency and stability with excellent results. Alternatively, particular systems characterized by an underlying network structure can be simulated by introducing more specific techniques based on a quantum-graph approach [17,34–41]. In this article, we apply the quantum-network approach to model the transport properties of mesoscopic spin interferometers subject to generic magnetic fields and RSOC by considering different geometries. The geometry of the interferometer is a key element since the carriers’ spin dynamics and the corresponding spin-phase gathering are sensitive to it [17,39–42]. Additionally, we propose a nontrivial extension of the quantum-network approach by considering the presence of 2469-9950/2021/103(15)/155419(13) 155419-1 ©2021 American Physical Society
A. HIJANO et al. PHYSICAL REVIEW B 103, 155419 (2021) in-plane Zeeman fields. We treat those in a similar way as the RSOC, however, they break time-reversal symmetry and, as a consequence, the wave function describing each edge of the quantum-network cannot be written in a compact form as in the case of flux of a magnetic field [43]oraRSOC[39]. The work is motivated by the experiments performed by Nitta’s group [19–22] showing evidence of electronic spin manipulation by geometric means in Aharonov-Casher interferometry. These experiments were done by using two-dimensional arrays of 40 ×40 ring and square interferometers, facilitating the measurement of a self-averaged conductance: The presence of multiple but small imperfections in the individual ring and square geometries lead to a universal signal that is independent of those details. One experiment revealed the manipulation of the geometric spin phase independently of the dynamical spin phase in Rashba rings [20]. More recently, topological spin-phase transitions in polygonal Rashba circuits have been reported [22]. By employing a quantumnetwork model, we reproduce the main results found in those experimental settings. Our approach provides a full quantum mechanical solution for the propagation of spin carriers inside the polygonal structure. The main strengths of our approach are the following: (i) we accounted for all possible propagating paths; (ii) there are no particular constraints imposed on the scattering matrix at the injector and collector nodes. Moreover, we take some steps forward and identify novel interferometric characteristics by proposing a field-texture engineering. This results in a physical situation similar to the spin-helix effect arising in systems subjected to Rashba and Dresselhaus spin-orbit couplings (SOCs) [44–46]. We also cross-check the results of our quantum-network approach by performing corresponding numerical simulations on tightbinding models. The paper is organized as follows. In Sec. II we take a quantum-network approach to model a one-dimensional circular loop as a regular polygon with a large number of vertices by following the method described in Ref. [41]. We generalize the method by introducing additional in-plane Zeeman fields beyond the perturbative approximation [20]. In Sec. III we derive the conductance as a function of the RSOC and Zeeman-field strengths and compare the obtained results to the experimental data and perturbative methods. Furthermore, we discover the occurrence of the transition line for which the Zeeman and Rashba terms cancel each other out and we study the effects on transport properties. We devote Sec. IV to compare the results obtained by the quantum-network method with those obtained by using a numerical tight-binding approach in the cases of clean and disordered systems. We present a short summary in Sec. Vwhere we analyze the strengths of the quantum network approach. In the Appendix we propose a technical derivation of one of the major analytical results of this work. II. MODEL AND FORMALISM We study the transport properties of ring-like structures by employing the formalism of quantum networks. We focus on regular polygons and approximate ring geometries as polygons with a large number of edges—see Figs. 1(a) to 1(d).In general terms, a metric network (or graph), is a collection of FIG. 1. Sketch of the polygonal structures that we consider for the quantum transport: (a) square, (b) hexagon, (c) octagon, (d) ring. In panels (e) and (f) we show the square and the ring of the discretized tight-binding version that we use in Sec. IV. The inset shows a zoom-in of the Yjunction between the incoming lead and one of the vertices of the square. nodes (or vertices), connected by edges (or one-dimensional intervals) of specified lengths [47]. In the graph terminology, regular polygons are also known as 2-regular graphs [38]. A quantum network is a metric graph equipped with a Schrödinger operator [43,48]. Thewavefunctionofthe quantum network satisfies boundary conditions at the vertices, which ensure the continuity (uniqueness) of the wave function and the conservation of the probability current. The fulfillment of these boundary conditions guarantees that the resulting Schrödinger operator is Hermitian [35,36,43]. We note in passing that this condition can be relaxed to account for non-Hermiatian Hamiltonians with PT -symmetry [49]. The continuity condition implies that the wave function assumes a certain value at a vertex, regardless of the bond from which it is approached. The concept of extended normal derivative must be introduced to apply the second boundary condition, whose definition might vary depending on the differential operator, i.e., it depends on the presence of a magnetic field or a SOC. To satisfy the current conservation condition, the sum of the outgoing extended derivatives at each vertex must vanish [35,38]. An extension for studying the n-particles quantum statistics has been proposed in Ref. [50]. In the following subsections, we consider a quantum network composed of single-mode quantum wires (QWs) subject to RSOC and to magnetic fields. In each case, we define a different Schrödinger operator (Hamiltonian) and the corresponding extended derivative. We start by introducing different spin-dependent Hamiltonians for the QWs composing the quantum network. Each Hamiltonian will be solved by using a spinorial plane-wave ansatz of the following form: =eikrχA χB,(1) where χA/Bare the two components of the spinor, kis the electronic momentum, and ris the local coordinate along the QW. A. Case of RSOC and magnetic flux We start by considering a QW in the xy-plane that points along the direction ˆ γ=(cos γ,sin γ,0). The QW is subject to RSOC and a weak magnetic field perpendicular to the xy-plane that interacts with the spin carriers only through minimal coupling (i.e., no Zeeman coupling) [39,40]. The 155419-2
QUANTUM NETWORK APPROACH TO SPIN … PHYSICAL REVIEW B 103, 155419 (2021) wire Hamiltonian reads ˆ H=1 2m∗(p+eA)2+¯hkR m∗[(p+eA)׈ z]·σ,(2) where kRis the coupling constant of the RSOC (in inverselength units), ˆ zis the unit vector along the z-axis, σis the vector of the Pauli matrices describing the electron spin, and m∗is the electron effective mass. The RSOC strength kRis related to the spin precession length LSO by LSO =π/kR.The wave function of the QW, fulfilling the Dirichlet boundary condition, can be written as a function of the values that the wave function takes at its vertices αand β[39,40]: (r)=e−iϕ(r)e−i(ˆ γ׈ z)·σkRr sin(k)[sin k(−r)α +sin (kr)eiϕ()ei(ˆ γ׈ z)·σkRβ],(3) where is the length of the QW, ris the local coordinate along the QW measured from vertex α, and the momentum k is related to the energy as k=√2m/¯h2+k2 R. The spinors αand βare the values of the wave function at the vertices αand β, respectively. In Eq. (3), we introduced a U(1) phase factor e−iϕ(r)related to the magnetic field via the vector potential A ϕ(r)=2π φ0r α dr·A(r),(4) where φ0=h/eis the flux quantum. This phase eventually leads to the Aharonov-Bohm (AB) effect [12,23]inclosed loops. The expression in Eq. (4) is proportional to the circulation of the vector potential between vertex αand point r [37,43]. The second phase factor in Eq. (3) is a SU(2) phase due to the RSOC. In closed loops it leads to the AharonovCasher (AC) effect [24] (electromagnetic dual of the AB effect) arising from the spin precession driven by the Rashba field [39,40,51]. The probability current corresponding to Hamiltonian (2)is j=−i¯h 2m∗†∂ ∂r−∂† ∂r+2ie ¯h(ˆ γ·A)† +2ikR†[(ˆ γ׈ z)·σ].(5) This expression hints that the probability current is not conserved by the continuity of the derivative of the wave function. However, the continuity of the extended derivative ∂ ∂r→D=∂ ∂r+ie ¯hˆ γ·A+ikR(ˆ γ׈ z)·σ(6) does ensure the conservation of the probability current. Once the wave function of all QWs is written as in Eq. (3), the conservation of probability current using the extended derivative is imposed at the vertices. Solving the resulting system of equations provides the value of the spinors at all the vertices α, and (r) by extension. B. Case of RSOC and Zeeman field We now consider a QW subject to RSOC and to an in-plane Zeeman field pointing in the direction ˆ α, where FIG. 2. Energy spectrum as a function of momentum for kSO =0 (left) and B=0 (right). In the left panel, Bis the pseudogap opened by the Zeeman field at zero momentum. The four propagating states at fixed energy are labeled by kf/b ±. B=B(cos α, sin α,0). The system Hamiltonian reads ˆ H=p2 2m∗+¯hkR m∗(p×z)·σ+μB·σ,(7) with μthe Bohr magneton. Unlike the RSOC term, the Zeeman term does not depend on momentum and thus it breaks time-reversal symmetry. Using the spinorial wave-function ansatz of Eq. (1), the Hamiltonian can be cast into the following matrix: ˆ H=¯h2k2 2m∗M∗ M¯h2k2 2m∗,(8) with M=(μBcos α+¯h2kRk msin γ)+i(μBsin α−¯h2kRk m cos γ).Thematrix(8) has the following eigenvalues and eigenvectors: ±=¯h2k2 2m∗±|M|,(9) |v±= 1 √2e−iθ/2 ±eiθ/2,(10) with θthe argument of M. The eigenvectors |v±lie within the xy-plane and remain constant along the wire. The energy spectrum of the quantum wire is given by Eq. (9), and consists of two energy bands due to the spin splitting induced by the RSOC and Zeeman interactions. The energy bands for the two limiting cases (kR=0 and B=0) are shown in Fig. 2. It is common knowledge that the dispersion relation in the presence of a Zeeman field is shifted vertically for opposite spins, while the RSOC introduces a horizontal shift [51]. In general, the interplay between both fields results in a more complex spectrum. The method described in this section is valid when the Fermi energy EFlies above the pseudogap B=2μ|B|, namely, the splitting induced by the Zeeman field at k=0. In this situation, there are four available propagating states for a given energy, two forward and two backward. We label the momenta and arguments corresponding to the four states as kf/b ±and θf/b ±, respectively. The superscript f/b indicates forward/backward propagation and the subscript ±indicates the energy band. A state with a defined propagation direction 155419-3
A. HIJANO et al. PHYSICAL REVIEW B 103, 155419 (2021) can be written as (r)=ˆ Rei¯ kr(0) .(11) Here we introduced the spin evolution matrix ˆ Rrelating the value of the wave function at point rto its initial value at r= 0. We find an analytic formula for the spin evolution matrix, given by [see the Appendix for its derivation] ˆ R=1 cos θ 2cos kr−θ 2ie−i¯ θsin kr 2 iei¯ θsin kr 2cos kr+θ 2.(12) For the sake of simplicity, we suppressed here the superscripts f/b. Additionally, we introduced the elements ¯ k= k++k− 2,k=k+−k−,¯ θ=θ++θ− 2, and θ =θ+−θ−.Note that, in general, these four quantities will be different for states propagating forward or backward. Equation (12) is one of the original results of this work since it allows for the exact treatment of hybrid RSOC and Zeeman fields within the quantum network method. In general, the wave function of a QW will be a linear combination of the available counterpropagating waves (r)=f(r)+b(r) (13a) =ˆ Rfei¯ kfrf(0) +ˆ Rbei¯ kbrb(0) .(13b) The spinors f(0) and b(0) are unknown constants that are fixed by applying the boundary conditions. When the Zeeman field is zero, the forward and backward elements satisfy the relations ¯ kb=−¯ kf,kb=−kf, ¯ θb=¯ θf+π, and θf=θb=0. After rearranging f/b(0) in terms of (0) and (), the wave function can be written as (r)= ˆ R(r) sin(k)[sin k(−r)(0) +sin (kr)ˆ R−1()()] ,(14) where now the spin evolution matrix ˆ Rcoincides with the SU(2) phase factor in Eq. (3). When the RSOC is zero and we have only the Zeeman term, which breaks time-reversal symmetry, we can still express the wave function with a structure similar to Eq. (13b), with the spin rotation matrix that now reads ˆ R(r)=eiˆα·σk 2r.(15) We note that a crossing of the energy band occurs when the Zeeman field is perpendicular to the wire and its modulus reaches to the critical value B=¯h2kkR mμ. Under this condition, the effective magnetic field created by the RSOC cancels with the in-plane magnetic field, so the only contribution to the energy comes from the kinetic term. This situation is similar to the spin-helix effect arising in systems with Rashba and Dresselhaus SOCs of equal strength [44–46]. The effective magnetic field due to the spin-fields vanishes for a certain momentum, so the Hamiltonian becomes spin-independent and an energy band crossing occurs. In this case, M=0, so the angles θ±for the two-fold degenerate solutions are not defined. A careful analysis shows that the spin evolution matrix is equal to the identity matrix. This comes as no surprise since the SU(2) terms in the Hamiltonian cancel each other out. Therefore, the spatial evolution of the state is simply given by the dynamic phase factor eikr that arises from the kinetic term. Equations (12) and (13) are the key step to generalize the quantum network method when an in-plane Zeeman field is applied. Boundary conditions are then applied at the vertices of the wire to obtain f/b(0), and (r) by extension. The Zeeman term does not contribute any additional term to the extended derivative, so it is given by Eq. (6) with A=0. C. Formalism for quantum transport To study the transport properties of quantum networks, we attach semi-infinite input and output leads to the vertices of the network [37,39,41]. Each lead consists of a single-mode QW with two spin channels [52]. The leads are not subjected to any interaction, so they are characterized at zero temperature by a wave vector kand a Fermi energy EF=¯h2k2/2m.We assume that the leads are connected to uncorrelated reservoirs, so that there are no phase relationships among electrons in different channels [53]. In a system with Nin (Nout) input (output) channels, if an electron is injected through input channel σwith wave number k, the wave function alongside the channels can be written as in,σ(r)=eikrδσσ+rσσe−ikr,(16a) out,σ (r)=tσσeikr,(16b) where ris the position measured from the edge (negative for input leads and positive for output leads). Here, rσσand tσσ are the channel-resolved reflection and transmission amplitudes, respectively. The indices σand σspecify both the lead and the spin state of the channel. We define the total transmission and reflection coefficients of a channel σas [16,51] Tσ= σ|tσσ|2,(17a) Rσ= σ|rσσ|2,(17b) where the sum runs over the input channels. The total transmission (reflection) is given by the sum of the transmission (reflection) coefficients of the output (input) channels T= σ Tσ= σσ|tσσ|2,(18a) R= σ Rσ= σσ|rσσ|2.(18b) The probability conservation (unitarity of the scattering matrix) imposes that T+R=1. The zero-temperature conductance Gbased on the Landauer formula reads [32] G=e2 hTr [tt†]=e2 hT.(19) It is clear from the previous expression that the conductance is bounded by the number input channels, such that G⩽ Nine2/h. 155419-4
QUANTUM NETWORK APPROACH TO SPIN … PHYSICAL REVIEW B 103, 155419 (2021) The derivatives of the wave function in the leads must also be taken into account when imposing the conservation of probability current. In an isolated quantum network, by imposing the continuity of the wave function and the conservation of the probability current we obtain a set of linear homogeneous equations where the variables are the values of the wave function at the vertices. This allows us to study the spectral properties of the quantum network via a secular equation [38,43]. When adding the external leads, the energy of the system is fixed by the Fermi energy of the leads EF. The transmission and reflection coefficients can be written in terms of the values of the wave function at the contacts. Due to the first term in the right-hand side of Eq. (16a), the set of equations becomes inhomogeneous, with a unique solution for T and R. If there is no Zeeman field, the wave function of the network is described by the values it takes at the vertices α[see Eqs. (3)]. For each input (output) lead there are two reflection (transmission) coefficients, one per spin channel. To satisfy the single-valuedness of the wave function at the vertices connected to external leads, one can write the reflection and transmission coefficients of the leads as a function of α. The number of variables of the problem is then equal to the number of vertices V. At each vertex the sum of the outgoing extended derivatives must be equal to zero, so there are V equations that impose the continuity of probability current. These equations fix the values of α, and consequently the reflection/transmission coefficients. Importantly, when the Zeeman field is finite, the wave function is described by spinors f αβ (0) and b αβ (0), which specify the wave function of a bond at one of its endpoints [see Eq. (13)]. The subscripts indicate that the QW is connected to vertices αand β. Together with the reflection/transmission coefficients, there are 2N+Next unknown variables, where N is the number of edges of the quantum network and Next is the number of input/output leads. For a vertex αconnected to Nαedges, we can write Nα−1 equations that impose the single-valuedness of the wave function. The total number of equations that verify the continuity of the wave function at the edges of quantum network are 2N+Next −V. In addition, at each vertex the sum of the outgoing extended derivatives must be equal to zero. In total there are 2N+Next equations that fix the values of the spinors and the transmission/reflection coefficients. For a generic vertex α, the continuity of the probability current reads α,β Dα,β (r)|r=0=0,(20) where the sum α,βruns over all vertices βwhich are connected to α. Equation (20) can be expressed in terms of f αβ (0) and b αβ (0) using Eq. (13b). In this case, the equation for the internal vertices is δ∈{f,b} α,β Mδ α,βδ α,β (0) =0.(21) In the case where the QW is subject to RSOC and a Zeeman field Mδ α,β =i¯ kδ+kδ 2tan θδ 2σz +ikδ 2 ˆ θδ cos θδ 2+kR(ˆ γ׈ z)·σ,(22) where ˆ θδ=(cos θδ,sin θδ,0). Consider a quantum network with a single input and output leads. If an electron with spin σis injected along the input lead, the equations for the external vertices read δ∈{f,b} α,β Mδ α,βδ α,β (0) =ikχσ−ik σ rσσχσ,(23a) δ∈{f,b} α,β Mδ α,βδ α,β (0) =−ik σ tσσχσ.(23b) The coefficients rσσand tσσcan be expressed as a linear combination of δ αβ (0) by applying the continuity of the wave function. Together with the equations that impose the continuity of the wave function of the internal edges, we obtain an inhomogeneous system of linear equations with 4N variables (two per spinor): The inhomogeneous term arises due to the first term on the rhs of Eq. (23a). The system can be solved numerically to obtain the value of the spinor of each bond at the local coordinate r=0. Once δ αβ (0) are obtained, it is straightforward to compute rσσand tσσ. Furthermore, Eq. (13b) provides the value of the wave function at any given point. In the case where the Zeeman term is zero, the boundary conditions for the leads reduce to the known cases in Refs. [37,39,40]: Mααα+ α,β Mαββ=0.(24) III. RESULTS In this section we study the transport properties of different polygons using the formalism we introduced in the previous section. We consider a series of regular polygons of constant perimeter Pwith an even number of vertices. Each polygon is connected to an input and an output field-free leads at opposite vertices | see Figs. 1(a) to 1(d). We evaluate the system conductance from the transmission probability applying the Landauer-Büttiker formalism [54] as dictated by Eq. (19). Taking the number of edges to infinity, the series of regular polygons converges to a circle, so we recover the conductance for a ring. For the case in which only RSOC is present, it was shown in Ref. [41] that this numerical procedure coincides with the analytical results for rings [55]. To match the conditions present in mesoscopic transport experiments, our numerical model must satisfy a series of constraints. The first one is the so-called semiclassical limit requiring the electronic wavelength to be much smaller than the system’s size. This condition can be written in terms of the 155419-5
A. HIJANO et al. PHYSICAL REVIEW B 103, 155419 (2021) FIG. 3. Average conductance Gkin units of 2e2/hfor various polygons: (a) square, (b) hexagon, (c) octagon, and (d) ring, subject to a magnetic flux φ/φ0and RSOC kRP/(2π). electronic wave number and the polygon’s perimeter as k2π P.(25) This limit justifies the interpretation of the system’s conductance in terms of carrier interference along classical-like propagating paths [56]. Moreover, it has been observed that slow carriers with smaller wave numbers are more prone to decoherence [20]. The wave number is also constrained by the size of the polygon’s edges. On the one hand, a polygonal geometry results noticed by the carriers on the condition that their wavelength is much smaller than the edges’ length, so that multiple wavelengths fit in one edge. Otherwise, the electron would not “see” the polygon’s vertices. On the other hand, in the specific case of ring modeling, the requirement is just the opposite: The wavelength must be much larger than the edges, instead, so that each vertex is hardly noticed by the carriers and the polygon can be interpreted as a ring k2πN P=2π L,(26) where Nis the number of edges of the polygon used to simulate the ring and Lis the length of each edge. Clearly, the larger the number of edges, the more fit the ring’s polygonal model. Moreover, for similar reasons, the spin precession length LSO should be much longer than edges as well [57]. A. Case of RSOC and magnetic flux Let us begin by discussing the transport properties of polygons subject to magnetic flux and RSOC. We present in Fig. 3the average conductance Gkfor different polygons. The average, performed over a small k-window around the Fermi wave number kFof incoming carriers, smooths out the energy-dependent oscillations of the conductance due to Fabry-Pérot-like interference [39,55]. This reproduces the situation found in low-(but-still-finite)-temperature transport experiments. The simulations of ring geometries are carried out by using polygons with 100 edges. The results presented in Fig. 3are a perfect example for highlighting the difference between an Abelian and a nonAbelian gauge field due to the orbital magnetic field and the RSOC, respectively. The conductance shows periodic AB oscillations, where the period is the flux quantum φ0for all the polygons. The maxima correspond to the constructive quantum interference of the electrons traveling through different paths. For example, in the Rashba field-free limit, the constructive interference occurs for integer multiples of the flux quantum. The AB phase acquired by an electron when moving around the polygon is 2πφ/φ0. Adding the contributions of all the possible paths gives rise to the interference pattern. The phase acquired by a particle moving through the shortest possible paths (clockwise and counterclockwise paths) will have the same magnitude, but opposite sign. For integer multiples of the flux quantum, the phase difference between the two paths is an integer multiple of 2πresulting in a constructive interference. However, the conductance is not exactly 2e2/h. The longer paths will also contribute to the transmission amplitude, each of which have a different dynamical phase. On the other side, for half integer multiples of the flux quantum, the contribution of the two opposite paths to the transmission amplitude are in counterphase, so the conductance drops to zero. The RSOC modifies the phase acquired by the electrons when traveling through the polygon; this leads to a shift of the position of the conductance maxima with respect to the magnetic flux. For instance, at kRP=2πthe conductance maxima appear at half integer multiples of φ0for all polygons, while the conductance vanishes for integer multiples of the flux quantum. The additional phase arises form the electron spin precession around the effective magnetic field arising from the RSOC, i.e., it acquires a non-Abelian SU(2) phase resulting in the Aharonov-Casher effect [24]. The spin-phase gathering is controlled by two different scales: The perimeter and the edge lengths. This is reflected on the oscillations of the conductance, which show broader and narrower maxima for different values of kRPassociated to two different frequencies [41]. The periodicity of the broader maxima is related to the edge lengths, where the period is Nπ. This period tends to infinity as the number of edges tends to infinity, so the broad maxima disappear for the ring, apart from the one located at the origin. The periodicity of the narrow maxima is related to the length of the perimeter, therefore, it has a weaker dependence on the number of edges of the polygon. The quasiperiod ranges from 4πfor the case of the square to 2πas the number of edges and the RSOC strength increase. Oscillations of period 2πare identified with the adiabatic limit: When the 155419-6
QUANTUM NETWORK APPROACH TO SPIN … PHYSICAL REVIEW B 103, 155419 (2021) FIG. 4. Average conductance Gkin units of 2e2/hfor α=0 for various polygons: (a) square, (b) hexagon, (c) octagon, and (d) ring. The dashed line corresponds to the critical line where BSO =B. dimensionless RSOC tends to infinity, we obtain the adiabatic limit in which the spin is aligned with the effective magnetic field during transport and Berry phases arise [41,55]. Adiabatic spin transport is never really achieved in polygons, where vertices act as spin-scattering centers due to the abrupt change of direction of the RSOC at the vertices of polygons. The results of Figs. 3(a) and 3(d) show a qualitative agreement with the experimental observations in ring [19,25,58] and square structures [42]. Still, a full agreement of the magnetoconductance periodicities require the introduction of disorder since the experiments present a periodicity halving due to the Altshuler-Aronov-Spivak (AAS) effect, a manifestation of the AB effect in the presence of dominant time-reversed-paths interference. [59] Such a periodicity halving will be reproduced in Sec. III C by implementing a numerical model for disorder. B. Case of RSOC and Zeeman field In this section we study the interplay between Zeeman and AC phases using the method described in Sec. II B. The quantum wires of the network are subject to RSOC and an in-plane Zeeman field, which breaks time-reversal symmetry. The averaged conductance for different polygons is shown in Fig. 4. The dashed line represents the critical line, the points where the applied Zeeman field is equal in magnitude to the effective magnetic field created by the RSOC, BSO =¯h2kkR mμ, which can be obtained from direct comparison between the second and third terms in Eq. (7). The dimensionless RSOC and Zeeman couplings are given by kRP/(2π) and mμBP/(2πk¯h2), respectively. For rings, Fig. 4(d), the AC oscillations shift to weaker values of the SOC field as the applied Zeeman field increases. These results are qualitatively consistent with the conductance shift observed experimentally by Nagasawa et al. in InGaAsbased quantum ring arrays, attributed to a geometric-phase manipulation [20]. However, in the experiment the periodicity of the magnetoresistance oscillations is halved due to the AAS effect. We fully recover this halving by introducing disorder | see Sec. III C. The RSOC field BSO is radial to the ring, while the inplane Zeeman field is homogeneous. Both fields lie on the xy plane, so the solid angle subtended by the magnetic field in parameter space corresponding to the Berry phase depends on whether the total magnetic field encircles the origin or not [60]. For simplicity, the Zeeman field is applied along the direction of the positive x-axis. For B<BSO, the solid angle is =2π, corresponding to a Berry phase π. However, for B>BSO the solid angle vanishes, so that the Berry phase is 0. The topology of the field texture, which coincides with the spin-eigenstate texture in the adiabatic limit, changes when the critical line is traversed. The results in Fig. 4show that the effects of this transition manifest in the conductance oscillations even in a nonadiabatic regime—small kRP/(2π). Strongly nonadiabatic spin textures allow for a transition of the topological properties of the spin eigenmodes when an in-plane Zeeman field is applied. These properties are characterized by the winding parity of the spin eigenmodes [22]. As it has been stated, for the ring this topological transition occurs when the applied Zeeman field is equal to the effective spin-orbit field. However, the AC oscillations for polygons with a finite number of edges show a sign reversal for much lower values of the Zeeman field. Figure 4shows the conductance for a Zeeman field direction α=0. However, the conductance pattern shows a strong dependence of αfor intermediate values of B. While the ring has a continuous rotational symmetry, polygons only remain invariant under rotations of an integer multiple of 2π/N.In addition, they have Nsymmetry planes, as well as inversion symmetry. The input and output leads break the rotational symmetry of polygons. Numerical calculations show that the only remaining symmetry planes are the horizontal and vertical planes. Therefore, the conductance will be the same for angles α,α=−α, and α =π−α. Introducing elastic disorder to the system removes these symmetry planes, although the inversion center remains, so that the conductance is the same for αand α =α+π. The conductance of a square for two orientations of the Zeeman field is shown in Fig. 5. For small values of the Zeeman field strength, the RSOC field contributes the most to the total magnetic field, so the oscillation pattern is almost identical in both cases. In the small RSOC limit, the conductance is also very similar for both orientations: For kR=0, the total magnetic field is equal to the applied Zeeman field, so it is homogeneous along the ring. The only effect on the energy spectrum is the splitting of the energy bands into two parabolas with opposite spin direction (see Fig. 2). The phase acquired by the electrons following the two shortest possible paths (the direct clockwise and counterclockwise paths) is the 155419-7
A. HIJANO et al. PHYSICAL REVIEW B 103, 155419 (2021) FIG. 5. Average conductance Gkof a square for a Zeeman field with an orientation of (a) α=0and(b)α=π/4. (c) Total magnetic field in a square for direct clockwise and counterclockwise (first row) paths and time-reversed (second and third rows) paths when BSO =Band α=π/4. The green arrows represents the Zeeman field, the purple ones the field associated to the RSOC, and the yellow ones the effective field due to the combination of Zeeman and RSOC. same, although the contribution of the longer paths results in the interference effect that gives rise to the oscillatory effect. The main difference between Figs. 5(a) and 5(b) is found around the critical line, where the oscillations of the conductance for α=π/4 are smoothed, see Fig. 6(a). As explained in Sec. II B, the energy bands of a wire become degenerate when the Zeeman and RSOC strength are the same and the Zeeman field is perpendicular to one of the edges of the polygon. The RSOC field is perpendicular to the motion of the electron, so in some edges, it cancels with the applied Zeeman field. For α=π/4, the Zeeman field is perpendicular to two opposite edges of the square, as it can be seen in Fig. 5(c). Therefore, electrons with any spin orientation propagating along these edges will not precess, and the interference effect between the upper and lower paths will be mitigated. In addition, the total magnetic field along the remaining two edges is the same, so the phase acquired by electrons following the direct clockwise and counterclockwise paths is the same. Higher-order contributions, due to paths that go several times around the polygons, are responsible for the nonconstant conductance along the critical line. The conductance along the critical line for several values of αisshowninFig.6. For the square, as αapproaches the α=π/4 direction, the oscillations become less pronounced. FIG. 6. Average conductance Gkas a function of the direction of the Zeeman field αalong the critical line for the square (a) without disorder and (b) with disorder. The disorder is implemented so as explained in Sec. III C. Disorder decreases the average conductance due to the random value of the dynamical phase. The conductance traces are vertically shifted of a constant 0.2 factor for clarity. Moreover, the oscillations show a more regular pattern, with a steadily increasing amplitude. Similar effects of mitigation of the spin procession due to RSCO are present in polygons with larger number of edges as well. However, the oscillatory pattern for the corresponding values of αdo not resemble the regular pattern obtained for the square. For a fixed perimeter P, as the number of edges of the polygon increases, the length of the edges become smaller, so the edge where the spin does not process has a smaller contribution towards the interference. C. Disordered case In this section, we show how disorder affects the results we presented in the previous sections. In general, disorder is inevitable in nanostructures and we need to account for its effects. Within the quantum network formalism, disorder can be introduced in several ways, e.g., randomly distributed pointlike scatterers, or more generally, the random elastic scattering matrix along the edges. We implement disorder following the scheme proposed in Refs. [37,39–41]: To simulate arbitrary shifts of the wave-function phase we implement random fluctuation of the length of each edge while preserving the orientation of the edges and keeping the perimeter Pof the polygon constant. We introduce therefore a length fluctuation parameter δ. These fluctuations account for the geometric imperfections present in experiments with arrays of rings and squares [19–22]. In the following we will focus on the case kδ ∼1, which can be reached in the semiclassical regime without a sizable modification of the loops’ areas such that the periodicity with respect to the magnetic flux is preserved [37]. Moreover, we introduce an additional energy average as done in the disorder-free case to boost numerical convergence. Contrary to the standard Anderson-like disorder, this model of elastic disorder in a single-loop quantum network will not produce a wave-function localization, but will lead to a reduction of the amplitude of oscillations of the average conductance. We will show that one of the main effects of disorder is to double the period of the oscillations of the average conductance of the system, and to lift the complete destructive interference [37,40,41]. The doubling of the period of oscillations corresponds to the so-called AAS oscillations [59] when considering the effect of the magnetic field or 155419-8
QUANTUM NETWORK APPROACH TO SPIN … PHYSICAL REVIEW B 103, 155419 (2021) FIG. 7. Average conductance Gk,δ as a function of the orbital magnetic field and of the RSOC in the presence of disorder for the cases of the square (upper row) and of the ring (lower row) obtained with the quantum network method. The three columns refer to different strengths of the length fluctuations: δ =5%, 10%, and 20%. AAS-like oscillations when considering the RSOC [19,58]. The emergence of the AAS oscillations in quantum networks with this type of disorder has previously been demonstrated by analyzing the Fourier amplitude of the conductance versus the magnetic flux in Ref. [37]. These results were in complete agreement with the experimental finding presented in Ref. [61]. Similar results were also presented in the presence of RSOC in oneand two-dimensional disordered quantum networks [39,40]. These quantum oscillations are dominated by the time-reversed paths [20,22]. For the sake of simplicity, in the following we present results for the case of disorder only considering the polygonal structures that are experimentally more relevant: The square and the ring—see Fig. 7for the case of AB and AC interference, and Fig. 8for the case of AC and Zeeman field. The results shown in Figs. 7and 8| especially those for δ =20%, to be compared to Figs. 3and 4, respectively | present a frequency doubling emerging from semiclassical time-reversed paths interference, which agree with the corresponding experimental findings for rings [19,20] and squares [22,42]. Additionally, by following the development of the interference pattern as the disorder strength increases, we further notice from Figs. 7and 8that the ring geometry appears to be less susceptible to show the frequency doubling (i.e., relatively stronger disorder is required by rings as compared to squares). This is likely due to the role played by the square vertices as spin-carrier scatterers. IV. VALIDATION OF THE QUANTUM NETWORK METHOD WITHIN THE TIGHT-BINDING APPROACH In this section we present results of a fully numerical approach, using a tight-binding model. We use KWANT,a PYTHON package facilitating tight-binding transport simulations [33]. The typical system we run simulations on are depicted in Figs. 1(e) and 1(f). We choose the units such that ¯h=m∗=e=1. The Hamiltonian for a square lattice with RSOC [62]is HRSOC =iλ 2a ic† iσxci+ˆy−c† iσyci+ˆx+H.c., (27) where λis the RSOC strength, ais the lattice size, c† i/ciare the creation/annihilation operators, and σi,i∈{x,y,z}are the Pauli matrices. The orbital magnetic field is implemented via a Peierls substitution t−→ teiϕ. Following the notation of the analytical section, the Hamiltonian for the Zeeman field is written as HZeeman =μ|B| 2a2 i c† ici(σxcos α+σysin α).(28) We stick to narrow systems here in order for the system to contain only a small number of energy bands (few modes). For calculating the average conductance we integrate over an energy window containing several level spacings, provided single-mode occupancy is observed. The results can be seen in Fig. 9, where the left block gives the results for the case including an orbital magnetic field and the right block is for the case including a Zeeman field. We find good qualitative agreement with the analytical results. Deviations from the analytical results can come from multiple sources. In the simulations we have to make a compromise between taking a thin wire, which can host only few modes, and a thicker wire, through which the electrons can move more easily without scattering. The results presented here have been run for an 155419-9